As others have said, to experience as many attractions as possible, go to the Fantasyland early in the morning. But for ambiance, revisit the land at night, and catch a ride on the carousel.
Something else to remember is that FL rides, like other darkrides, are often best seen at night when your eyes don't have to make a very big adjustment from the bright sunlight to the dark.
I've always found Fantasyland to be a place to see in the morning, when everything is pretty much visible. I get the same vibe with Mickey's Toontown.
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